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Electronic Light-Matter Strong Coupling in Nanofluidic Fabry-Pérot Cavities

Journal article
Authors H. Bahsoun
T. Chervy
A. Thomas
Karl Börjesson
M. Hertzog
J. George
E. Devaux
C. Genet
J. A. Hutchison
T. W. Ebbesen
Published in ACS Photonics
Volume 5
Issue 1
Pages 225-232
ISSN 2330-4022
Publication year 2018
Published at Department of Chemistry and Molecular Biology
Pages 225-232
Language en
Links doi.org/10.1021/acsphotonics.7b0067...
Keywords Chlorin e6, fluorescence lifetime decay, quantum yield, Rabi splitting, radiative and nonradiative decay rates, Emission properties, Fluorescence lifetimes, Nanoscale dimensions, Nonradiative decay rate, Solid molecular films, Strong-coupling regime
Subject categories Photonics

Abstract

Electronic light-matter strong coupling has been limited to solid molecular films due to the challenge of preparing optical cavities with nanoscale dimensions. Here we report a technique to fabricate such Fabry-Pérot nanocavities in which solutions can be introduced such that light-molecule interactions can be studied at will in the liquid phase. We illustrate the versatility of these cavities by studying the emission properties of Chlorin e6 solutions in both the weak and strong coupling regimes as a function of cavity detuning. Liquid nanocavities will broaden the investigation of strong coupling to many solution-based molecular processes. © 2017 American Chemical Society.

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